雷聖賓，男，博士，天津大學教授，博士生導師。
基本介紹
- 中文名：雷聖賓
- 職業：教師
- 學位/學歷：博士
- 專業方向：有機二維材料與器件
- 任職院校：天津大學
個人經歷,學術成果,研究方向,榮譽獎項,
個人經歷
1.教育經歷
1999/9-2002/7：中科院化學研究所，博士，物理化學，導師：王琛研究員
1996/9-1999/7：山東大學化學系，碩士，物理化學，導師：陳慎豪教授
1992/9-1996/7：山東大學化學系，本科
2.研究工作經歷
2015/8至今：天津大學，天津市分子光電科學重點實驗室，博士生導師
2009/9-2015/7：哈爾濱工業大學，微系統與微結構製造教育部重點實驗室，博士生導師
2006/7-2009/8:比利時魯汶天主教大學化學系，光化學與光譜實驗室，博士後
2005/1-2006/7:中國科學院化學研究所分子納米結構與納米技術院重點實驗室，副研究員
2002/7-2004/12:中國科學院化學研究所分子納米結構與納米技術院重點實驗室，助理研究員
學術成果
近年二維聚合物的形成機制和物理化學性質、表面限域的動態共價化學研究方面取得了一系列科研成果。提出了二維超分子格線的濃度控制和模板分子誘導策略，並成功將之套用於表面動態化學反應的調控，揭示了表面動態化學反應中的關鍵控制因素，初步實現了對動態共價反應從體相到界面的控制；發展了一種操作簡便、條件溫和的二維聚合物表面合成方法，實現了大範圍、連續、具有規整結構的系列二維聚合物的室溫製備；實驗結合理論計算研究了二維聚合物及其與石墨烯複合物的化學與能帶結構，探索了其在電化學儲能及光電感測方面的套用。
在Angew. Chem. Int. Ed., J. Am. Chem. Soc.,Nano Lett.,Adv. Mater.,ACSNano,Nanoscale,Chem. Comm.,Chem. Eur. J.等雜誌發表SCI收錄論文120餘篇，為Top.Curr.Chem., Chem. Soc. Rev.,Angew. Chem. Int. Ed., Nanoscale, Chem. Comm., CrystEngComm撰寫綜述六篇。
論文被引用4200餘次，其中近五年來被引用2000餘次。其中10篇論文單篇引用超過100次，第一作者論文單篇最高引用次數超過次。個人H因子34。獲2005年度中國化學會青年化學獎，2009年獲教育部新世紀優秀人才計畫支持。J. Am. Chem. Soc.,Nanoscale, Chem. Eur. J., Chem. Comm., Langmuir, Polymer, Soft Matter, ChemPhysChem, Sci. China Chem.等雜誌審稿人，比利時弗拉芒區基金(the research foundation Flanders)評閱人。《Transactions of Tianjin University》（即《天津大學學報（英文版）》）編委
主持或參加科研項目及人才基金項目情況
1. 國家自然科學基金委面上項目，21572157，席夫鹼二維聚合物的表面反應製備及性質研究，2016.1－2019.12，65萬，正在進行中，主持。
2. 國家自然科學基金委面上項目，21373070，石墨烯－有機半導體界面結構及結構與性能關係，2014.1－2017.12，82萬，已結題，主持。
3. 國家自然科學基金委面上項目，21173061，固液界面多孔分子格線的功能化， 2012.1－2015.12，61萬，已結題，主持。
4. 教育部新世紀優秀人才，2010.1-2012.12，50萬，已結題，主持。
5. 教育部留學歸國人員科研啟動基金, 2013.1-2015.12,3.0萬, 已結題，主持。
6. 校985領軍學者與團隊，2011.1-2012.12，32萬，已結題，主持。
7. 校基礎研究傑出人才培育計畫，2011.1-2012.12，18萬，已結題，主持。
8. 新型TiO2/石墨烯複合材料的製備及其催化機理研究，水資源與水環境國家重點實驗室開放課題，2011.7-2014.6，10萬，已結題，主持。
9. 國家自然科學基金委面上項目，50573089，導電高分子薄膜的結構與性能研究，2006.1－2008.12，26萬，已結題，主持。
10. 國家自然科學基金委面上項目（青年），20303023，多組分表面分子納米結構構築與表征，2004.1－2006.12，24萬，已結題，主持。
11. 國家納米中心協作實驗室課題，蛋白質生物納米感測器的研究，2004.7-2006.6， 50萬，已結題，參加。
12. 中科院知識創新工程重大項目，2002CCA0310，《若干納米器件的基礎性研究》子課題：納米結構的檢測與表征，2001.1-2005.12，100萬，已結題，參加。
13. 基金委面上項目，20073053，有機分子的可控吸附與組裝的掃描探針顯微研究，2001.1－2003.12，25萬，已結題，參加。
14. 科技部973項目，G2000077501，973《創造新物質的分子工程學研究》子課題：單分子和納米基元的結構研究，2000.9-2005.9，133萬，已結題，參加。
近五年論文
2018
1. Chunhua Liu, Eunsol Park, Jie Liu, Yanxia Yu, Yinghua Jin, Wei Zhang*, Shengbin Lei*, Wenping Hu, Surface-Confined Dynamic Covalent System Driven by Olefin Metathesis
Angew. Chem. Int. Ed.2018,57(7), 1869-1873.
2. Chunhua Liu,Eunsol Park, Jie Liu, Yanxia Yu, Yinghua Jin, Wei Zhang*, Shengbin Lei*, Wenping Hu, Effective Separation of Arylenevinylene Macrocycles with a Surface Confined Two-Dimensional Imine Covalent Organic Framework,
Angew. Chem. Int. Ed.2018,DOI: 10.1002/anie.201803937.
3. Chunhua Liu, Ling Yang, Yan Wang, Shengbin Lei*,Substrate effects in the supramolecular assembly of 2,4,6-tris(4-bromophenyl)-1,3,5-triazine on graphite and graphene
J. Phys. Chem. C,2018,10.1021/acs.jpcc.8b02979.
4. Jiang Sun, Shengbin Lei, Guest-Induced Structural Transformation and Its Effect on the Redistribution of the Surface Confined Combinatorial Libraries
J. Phys. Chem. C,2018, 10.1021/acs.jpcc.8b03215.
5. Yanxia Yu, Nerea Bilbao, Lander Verstraete, Shengbin Lei*, and Steven De Feyter,* The impact of grafted surface defects on the on-surface Schiff-base chemistry at the solid-liquid interface
Chem. Commun.2018,Submitted.
6. Zongxia Guo,* Ping Yu, Kai Sun, Shengbin Lei, Yuanping Yi and Zhibo Li*, Role of halogenhalogen interactions in the 2D crystallization of n-semiconductors at the liquid–solid interface
Phys. Chem. Chem. Phys., 2018, 19(47), 31540-31544.
7. Yumin Chen, Ke Deng*, Shengbin Lei, Rong Yang, Tong Li, Yuantong Gu, Yanlian Yang*, Xiaohui Qiu*, Chen Wang, Single-molecule Insights into Surface-mediated Homochirality in Hierarchical Peptide Assembly
Nature Comm., 2018, accepted.
2017
8. Yanxia Yu, Chunhua Liu, Jiang Sun, Shengbin Lei*, DynamicCovalentChemistry ofImine Polymers at Liquid/solid Interfaces Investigated by Scanning Tunneling Microscopy
RSC Advances,2017,7, 11496 - 11502.
9. Jiang Sun,Yanxia Yu, Chunhua Liu, Shengbin Lei*,Surface- and Guest-Promoted Product Selection from a Dynamic Covalent Library: A Scanning Tunneling Microscopic Study
J. Phys. Chem. C, 2017,121, 3437-3444.
10. Yanxia Yu, Ya li Zheng,Shengbin Lei*, From a Two-Dimensional Supramolecular Network to One-Dimensional Covalent Polymer at the Liquid/Solid Interface: Insight into the Role of the Stoichiometric Ratio of the Precursors
J. Phys. Chem. C, 2017,121 (1), 593-599.
2016
11. Chunhua Liu, Wei Zhang, Qingdao Zeng, Shengbin Lei*,A PhotoresponsiveTwo-Dimensional CovalentOrganicFramework: Surface-Confined Synthesis, Isomerization and Controlled Guest Capture and Release
Chem. Eur. J.2016,22, 6768-6773.
12. Lirong Xu, Yanxia Yu, Jianbin Lin, Xin Zhou,* Wei Quan Tian,Damian Nieckarz, Pawel Szabelski,*Shengbin Lei,*On-Surface Synthesis of Two-dimensional Imine Polymers with Tunable Band Gap: a Combined STM, DFT and Monte Carlo Investigation
Nanoscale,2016,8, 8568 - 8574.
13. Yanxia Yu, Jianbin Lin, Yan Wang, Qingdao Zeng, Shengbin Lei,* Room Temperature On-Surface Synthesis of Crystalline Two-Dimensional Imine Polymers at the Solid/Liquid Interface: Concentration Takes Control
Chem. Comm.,2016,52, 6609-6612.
14. Jiang Sun, Xin Zhou* and Shengbin Lei*, Host-Guest Architectures with a Surface Confined Imine Covalent Organic Framework as Two-Dimensional Host Networks
Chem. Comm., 2016,52, 8691-8694.
15. Yanxia Yu, Ling Yang,*Chunhua Liu, Wei-Quan Tian,Yan Wang,* Shengbin Lei*, Hierarchical Construction of Cross-Junction of Molecular Wires with Covalent and Noncovalent Interactions at the Liquid/Solid Interface
Chem. Comm., 2016,52, 8317-8320.
16. Chunhua Liu, Yanxia Yu,Wei Zhang, Qingdao Zeng,Shengbin Lei*,Room Temperature Synthesis of Covalent Organic Frameworkswith Boronic Ester Linkage at the Liquid/Solid interface
Chem. Eur. J,2016,22, 18412-18418.
17. Jia Zhang, Chao Zhao, Na Liu, Huanxi Zhang, Jingjing Liu, Yong Qing Fu, Bin Guo, Zhenlong Wang*, Shengbin Lei, PingAn Hu*, Tunable electronic properties of graphene through controlling bonding configurations of doped nitrogen atoms
Scientific Reports, 2016,6, 28330.
2015
18. Lirong Xu, Lili Cao, Zongxia Guo,Zeqi Zha,Shengbin Lei*,Side-Functionalized Two-Dimensional Polymers Synthesized via On-Surface Schiff-Base Coupling
Chem. Comm.,2015,51, 8664 - 8667.
19. Xiu-Ling Sun, Li-Xia Fan, Yong-Jing Yang, Zongxia Guo*, Wei Quan Tian, Shengbin Lei*,Synthesis of One Dimensional Schiff Base Polymers Containing Oligothiophene Building Block on the Graphite Surface
Chem. -EurJ., 2015, 21, 6898-6905.
20. Xiuling Sun, Lixia Fan, Xin Zhou*, Wei Quan Tian, Zongxia Guo*, Zhibo Li,Xiaokang Li,Shengbin Lei*, SurfaceConfinedSynthesis of Porphyrin ContainingTwo-Dimensional Polymers: the Effect of Rigidity and Preferential Adsorption of Building Blocks
Chem. Comm., 2015,51, 5864-5867.
21. Xin Zhou, Longtao Jiang, Shengbin Lei*, Wei Quan Tian*, Gaohui Wu*,Micro-mechanism in Self-lubrication of TiB2/Al Composite
ACS Appl. Mater. Interfaces, 2015, 7, 12688−12694.
22. Zeqi Zha, Lirong Xu,Zhikui Wang, Qinmin Pan,Shengbin Lei*,3D Graphene Functionalized by Covalent Organic Framework Thin Film as Capacitive Electrode in Alkaline Media
ACS Appl. Mater. Interfaces, 2015,7 (32), pp 17837–17843.
23. Yanxia Yu, Jiang Sun, Shengbin Lei*,Surface Confined Synthesis of One-DimensionalSchiff Base PolymersInvestigated byScanning Tunneling Microscopy
J. Phys. Chem. C,2015, 119,16777–16784.
24. Yanqiu Jiang, Zongxia Guo, Shengbin Lei*,The Assembling of Poly (3-Octyl-Thiophene) on CVD Grown Single Layer Graphene
Scientific Reports, 2015,5, 17720; doi: 10.1038/srep17720.
25. Junyan Zhu, Zeyuan Dong*, Shengbin Lei, Lili Cao, Bing Yang, Wenfang Li, Yuanchao Zhang, Junqiu Liu*, and Jiacong Shen,Design of Aromatic Helical Polymers for STM Visualization : Imaging of Single and Double Helices with a Pattern of p –p Stacking
Angew. Chem. Int. Ed.,2015, 54(10), 3097-3101.
2014
26. Lirong Xu, Xin Zhou, Wei Quan Tian, Teng Gao, Yan Feng Zhang, Shengbin Lei,* and Zhong Fan Liu,Surface Confined Single Layer Covalent Organic Framework on Single Layer Graphene Grown on Copper Foil
Angew. Chem. Int. Ed.,2014, 53(36), 9564-9568.
27. Xiuling Sun, Youbing Mu, Jia Zhang, Xiaona Wang, Pingan Hu, Xiaobo Wan,* Zongxia Guo,* and Shengbin Lei*,Tuning Self-Assembly of Oligothiophenes on CVD Graphene: Effect of Functional Group, Solvent and Substrate
Chem. -Asian J., 2014, 9(7), 1888-1894.
28. Lili Cao, Lirong Xu, Dahui Zhao, Kazukuni Tahara, Yoshito Tobe, Steven De Feyter, Shengbin Lei*, Efficient Molecular Recognition Based on Nonspecific van der Waals Interaction at the Solid/Liquid Interface
Chem. Commun.2014, 50 (80), 11946-11949.
29. Min Li, Peng Xie, Ke Deng, Yan-Lian Yang, Sheng-Bin Lei, Zhong-Qing Wei,* Qing-Dao Zeng* and Chen Wang*, A dynamic study of the structural change in thebinary network in response to guest inclusion
Phys. Chem. Chem. Phys., 2014, 16, 8778-8782.
30. Kazukuni Tahara, Jinne Adisoejoso, Koji Inukai, Shengbin Lei, Aya Noguchi, Bing Li, Willem Vanderlinden, Steven De Feyter* and Yoshito Tobe*,Harnessing by a diacetylene unit: a molecular design for porous two-dimensional network formation at the liquid/solid interface
Chem. Commun.2014, 50,2831-2833.
31. Li Wang, Xingping Lu, Shengbin Lei and Yonghai Song*, Graphene-based polyaniline nanocomposites: preparation, properties and applications
J. Mater. Chem. A, 2014, 2, 4491-4509.
32. Liming Qin, Jie Zhao, Shengbin Lei, and Qinmin Pan*, A Smart “Strider” Can Float on Both Water and Oils,
ACS Appl. Mater. Interfaces, 2014, 6, 21355-2136.
2013
33. Lirong Xu, Xin Zhou, Yanxia Yu, Wei Quan Tian*, Jun Ma,Shengbin Lei*, Surface Confined Crystalline Two-Dimensional Covalent Organic Frameworksviaon Surface Schiff-Base Coupling
ACS nano, 2013, 9, 8066-8073.
34. Xiuling Sun, Jia Zhang, Xiaona Wang,Cuiyun Zhang, Pingan Hu,Youbing Mu, Xiaobo Wan, Zongxia Guo* andShengbin Lei*,“Oligothiophenes on CVDGrapheneGrown onMulti-crystallineCopperFoil: SupramolecularAssembling and Morphology Impact”
Chem. Commun.2013, 49, 10317-10319.
35. Lirong Xu, Liu Yang, Lili Cao, Tian Li, Shusen Chen, Dahui Zhao*,Shengbin Lei*, Jun Ma, “Effect of Bulky Substituent on the Self-Assembly and Mixing Behavior of Arylene Ethynylene Macrocycles at the Solid/Liquid Interface”
Phys. Chem. Chem. Phys., 2013, 15, 11748-11757.
36. Yong-Tao Shen, Ning-Bo Zhu, Xue-Mei Zhang,Shengbin Lei, Zhongqing Wei, Min Li,* Dahui Zhao,* Qing-Dao Zeng,* Chen Wang*，“Assemblies at the Liquid-Solid Interface: Chirality Expression from Molecular Conformers”
ChemPhysChem, 2013, 14, 92–95.
37. Xiaona Wang, Xiuling Sun, Ping An Hu,* Jia Zhang, Lifeng Wang, Wei Feng, Shengbin Lei, Bin Yang, and Wenwu Cao, Colorimetric Sensor Based on Self-Assembled Polydiacetylene/Graphene-Stacked Composite Film for Vapor-Phase Volatile Organic Compounds
Adv. Funct. Mater., 2013, 23, 6044-6050.
研究方向
1)有機二維材料與器件
致力於發展具有光電功能的有機二維材料，尤其是薄膜材料的製備技術，探索其在場效應電晶體、記憶存儲器件、光檢測器等領域的套用。
2) 表面限域的動態共價化學
在動態共價化學反應中表面限域作用不僅體現在對產物的選擇和放大作用，而且在二維聚合物的生長過程中范德華外延作用還可以誘導生成更加長程有序的結構。本研究方向主要致力於探索表面限域作用對動態共價體系的產物選擇和反應過程的新奇效應以及利用表面限域效應製備長程有序的二維聚合物材料。
榮譽獎項
獲2005年中國化學會青年化學獎
2009年獲教育部新世紀優秀人才計畫支持
